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The dynamics of single step hole transport processes from a guanine cation radical (G+·) to GG, GGG and deazaguanine (Z) secondary electron donors separated by one or two A:T base pairs have been investigated by means of nanosecond time-resolved absorption spectroscopy with kinetic modeling. Photoinduced electron transfer from G to a stilbenedicarboxamide (Sa) hairpin linker is used to generate a...
The dynamics of single step hole transport processes from a guanine cation radical (G+·) to GG, GGG and deazaguanine (Z) secondary electron donors separated by one or two A:T base pairs have been investigated by means of nanosecond time-resolved absorption spectroscopy with kinetic modeling. Photoinduced electron transfer from G to a stilbenedicarboxamide (Sa) hairpin linker is used to generate a...
The synthesis and properties of a perylenediamide diol linker and several DNA hairpins possessing this linker are described. The diol linker absorbs and fluoresces strongly in the visible. Hairpins having poly(dA)–poly(dT) stems have fluorescence quantum yields and decay times similar to those of the linker, indicating that hole injection does not occur from the singlet excited linker into the base...
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