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Optimization of the back contact interface is crucial for improving the performance of Cu2ZnSnS4 (CZTS) thin film solar cells. In this paper, self‐depleted CuSCN is deployed as an intermediate layer at the Mo/CZTS interface to improve the quality of the back contact. This CuSCN layer, obtained via aqueous solution processing, reduces the thickness of Mo(S,Se)2 and eliminates multi‐layer crystallization...
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