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In this work, it is reported that large‐area (centimeter‐scale) arrays of non‐close‐packed polystyrene‐tethered gold nanorod (AuNR@PS) can be prepared through a liquid–liquid interfacial assembly method. Most importantly, the orientation of AuNRs in the arrays can be controlled by changing the intensity and direction of electric field applied in the solvent annealing process. The interparticle distance...
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