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Ein genaues Verständnis der Faktoren, welche die Lumineszenzlebensdauer von Übergangsmetallverbindungen bestimmen, ist für Anwendungen in der Photokatalyse und der photodynamischen Therapie von entscheidender Bedeutung. Die im Falle von [Ru(bpy)3]2+ (bpy=2,2’‐Bipyridin) allgemein akzeptierte Theorie besagt, dass die Emissionslebensdauer durch Optimierung der Energiebarriere zwischen dem emittierenden...
Calculating temperature‐dependent emission lifetimes is like a scavenger hunt. In their Research Article (e202308803), Leticia González et al. show that in [Ru(bpy)3]2+, the pathway governed by the lowest 3MC‐trans excited state triplet minimum leads astray. Instead, through the concept of rate‐determining states and an extended kinetic model that takes all the different Jahn–Teller isomers into account,...
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