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Coiled coils (CCs) are powerful supramolecular building blocks for biomimetic materials, increasingly used for their mechanical properties. Here, we introduce helix‐inducing macrocyclic constraints, so‐called staples, to tune thermodynamic and mechanical stability of CCs. We show that thermodynamic stabilization of CCs against helix uncoiling primarily depends on the number of staples, whereas staple...
Coiled Coils (CCs) sind vielversprechende Proteinbausteine für biomimetische Materialien, die aufgrund ihrer mechanischen Eigenschaften vermehrt genutzt werden. In dieser Arbeit wurden Helix‐induzierende makrozyklische Klammern in ein CC‐Heterodimer eingefügt, um die thermodynamische und mechanische Stabilität dieses CCs zu erhöhen. Die thermodynamische Stabilisierung des CCs wird durch die Anzahl...
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