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Atomic Cl was generated by pulsed laser photolysis at 193nm of CCl 4 , and was monitored by time resolved resonance fluorescence in the course of reaction with excess C 2 H 2 , diluted in Ar bath gas at pressures from 13 to 800mbar. At 288K simple pseudo first order kinetics were observed. Over 365–430K bi-exponential decays were obtained, because of equilibration between the...
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