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Achieving strong adsorption and catalytic ability toward polar lithium polysulfide species (LiPSs) of the sulfur host in lithium–sulfur (Li–S) batteries is essential for their electrochemical cyclic stability. Herein, a strategy of “self‐termination of ion exchange” is put forward to synthesize the novel yolk‐shell sulfur host composed of ZnO nanoparticles confined in Co‐doped NiO (CDN) polyhedron...
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