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Bright supramolecular fluorescent organic nanoassemblies (FONs), based on strongly polar red‐emissive benzothiadiazole fluorophores containing acidic units, are fabricated to serve as theranostic tools with large colloidal stability in the absence of a polymer or surfactant. High architectural cohesion is ensured by the multiple hydrogen‐bonding networks, reinforced by the dipolar and hydrophobic...
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