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Tautomers of the nucleobases play fundamental roles in spontaneous mutations of DNA. Tautomers of neutral cytosine have been studied in the gas phase, but much less is known about charged species. Here, we report the observation and characterization of three tautomers of deprotonated cytosine anions, [trans‐keto‐amino‐N3H‐H8b] (tKAN3H8b−), [cis‐keto‐amino‐N3H‐H8a] (cKAN3H8a−) and [keto‐amino‐H] (KAN1...
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