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Molecules with large enough dipole moments can bind an electron by the dipole field, which has little effect on the molecular core. A molecular anion can be excited to a dipole‐bound state, which can autodetach by vibronic coupling. Autodetachment spectroscopy of a complex anion cooled in a cryogenic ion trap is reported. Vibrational spectroscopy of the dehydrogenated uracil radical is obtained by...
Dipol‐gebundene Zustände: Die Elektronenablösung aus schwingungsangeregten Dipol‐gebundenen Zuständen von Phenoxidionen wurde mit Photoelektronen‐Spektroskopie beobachtet. Das Bild zeigt die Wellenfunktion eines Dipol‐gebundenen Zustands und die beobachteten Normalschwingungen. Der blaue Orbitallappen weist darauf hin, dass das Elektron schwach an den Dipol gebunden ist.
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