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Sulfuryl fluoride (SO2F2) is of a fundamental interest due to its nearly tetrahedral symmetry, making it, thereby, an intermediate case between spherical and asymmetric-top molecules. It is also a widely-used insecticide and an atmospheric pollutant. A new high-resolution infrared spectrum of the (ν9,ν7,ν3) bending triad of SO2F2 in the 550cm−1 region has been recorded at 165K with a spectral resolution...
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