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Sulfide electrolytes with high ionic conductivity hold great promise for all‐solid‐state lithium batteries. However, the parasitic redox reactions between sulfide electrolyte and Li metal result in interfacial instability and rapid decline of the battery performance. Herein, a redox‐resistible Li6PS5Cl (LPSC) electrolyte is created by regulating the electron distribution in LPSC with Mg and F incorporation...
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