Search results for: Zhi-Ming Zhang

Items from 1 to 20 out of 158 results

article

Single Dispersion of Fe(H₂O)₂‐Based Polyoxometalate on Polymeric Carbon Nitride for Biomimetic CH₄ Photooxidation

Jing Ren, Baifan Wang, Hua‐Qing Yin, Peng Zhang, more

Advanced Materials > 36 > 31 > n/a - n/a

Direct methane conversion to value‐added oxygenates under mild conditions with in‐depth mechanism investigation has attracted wide interest. Inspired by methane monooxygenase, the K₉Na₂Fe(H₂O)₂{[γ‐SiW₉O₃₄Fe(H₂O)]}₂·25H₂O polyoxometalate (Fe‐POM) with well‐defined Fe(H₂O)₂ sites is synthesized to clarify the key role of Fe species and their microenvironment toward CH₄ photooxidation. The Fe‐POM can...

article

Single‐cluster Functionalized TiO₂ Nanotube Array for Boosting Water Oxidation and CO₂ Photoreduction to CH₃OH

Shen‐Yue Xu, Wenxiong Shi, Juan‐Ru Huang, Shuang Yao, more

Angewandte Chemie International Edition > 63 > 28 > n/a - n/a

Solar‐driven CO₂ reduction and water oxidation to liquid fuels represents a promising solution to alleviate energy crisis and climate issue, but it remains a great challenge for generating CH₃OH and CH₃CH₂OH dominated by multi‐electron transfer. Single‐cluster catalysts with super electron acceptance, accurate molecular structure, customizable electronic structure and multiple adsorption sites, have...

article

Single‐cluster Functionalized TiO₂ Nanotube Array for Boosting Water Oxidation and CO₂ Photoreduction to CH₃OH

Shen‐Yue Xu, Wenxiong Shi, Juan‐Ru Huang, Shuang Yao, more

Angewandte Chemie > 136 > 28 > n/a - n/a

article

Building Co₁₆‐N₃‐Based UiO‐MOF to Expand Design Parameters for MOF Photosensitization

Guang‐Chen Guo, Jiong‐Peng Zhao, Song Guo, Wen‐Xiong Shi, more

Angewandte Chemie International Edition > 63 > 27 > n/a - n/a

The construction of secondary building units (SBUs) in versatile metal–organic frameworks (MOFs) represents a promising method for developing multi‐functional materials, especially for improving their sensitizing ability. Herein, we developed a dual small molecules auxiliary strategy to construct a high‐nuclear transition‐metal‐based UiO‐architecture Co₁₆‐MOF‐BDC with visible‐light‐absorbing capacity...

article

Building Co₁₆‐N₃‐Based UiO‐MOF to Expand Design Parameters for MOF Photosensitization

Guang‐Chen Guo, Jiong‐Peng Zhao, Song Guo, Wen‐Xiong Shi, more

Angewandte Chemie > 136 > 27 > n/a - n/a

article

Water‐Mediated Selectivity Control of CH₃OH versus CO/CH₄ in CO₂ Photoreduction on Single‐Atom Implanted Nanotube Arrays

Juan‐Ru Huang, Wen‐Xiong Shi, Shen‐Yue Xu, Hao Luo, more

Advanced Materials > 36 > 9 > n/a - n/a

Controllable methanol production in artificial photosynthesis is highly desirable due to its high energy density and ease of storage. Herein, single atom Fe is implanted into TiO₂/SrTiO₃ (TSr) nanotube arrays by two‐step anodization and Sr‐induced crystallization. The resulting Fe‐TSr with both single Fe reduction centers and dominant oxidation facets (001) contributes to efficient CO₂ photoreduction...

article

Identification of Crucial Photosensitizing Factors to Promote CO₂‐to‐CO Conversion

Ping Wang, Song Guo, Qiu‐Ping Zhao, Shen‐Yue Xu, more

Angewandte Chemie International Edition > 63 > 7 > n/a - n/a

The sensitizing ability of a catalytic system is closely related to the visible‐light absorption ability, excited‐state lifetime, redox potential, and electron‐transfer rate of photosensitizers (PSs), however it remains a great challenge to concurrently mediate these factors to boost CO₂ photoreduction. Herein, a series of Ir(III)‐based PSs (Ir‐1–Ir‐6) were prepared as molecular platforms to understand...

article

Identification of Crucial Photosensitizing Factors to Promote CO₂‐to‐CO Conversion

Ping Wang, Song Guo, Qiu‐Ping Zhao, Shen‐Yue Xu, more

Angewandte Chemie > 136 > 7 > n/a - n/a

article

Spin Manipulation in a Metal–Organic Layer through Mechanical Exfoliation for Highly Selective CO₂ Photoreduction

Dayu Wu, Hua‐Qing Yin, Zeshi Wang, Mingren Zhou, more

Angewandte Chemie International Edition > 62 > 18 > n/a - n/a

Spin manipulation of transition‐metal catalysts has great potential in mimicking enzyme electronic structures to improve activity and/or selectivity. However, it remains a great challenge to manipulate room‐temperature spin state of catalytic centers. Herein, we report a mechanical exfoliation strategy to in situ induce partial spin crossover from high‐spin (s=5/2) to low‐spin (s=1/2) of the ferric...

article

Spin Manipulation in a Metal–Organic Layer through Mechanical Exfoliation for Highly Selective CO₂ Photoreduction

Dayu Wu, Hua‐Qing Yin, Zeshi Wang, Mingren Zhou, more

Angewandte Chemie > 135 > 18 > n/a - n/a

article

Co‐Dissolved Isostructural Polyoxovanadates to Construct Single‐Atom‐Site Catalysts for Efficient CO₂ Photoreduction

Yu‐Jie Wang, Gui‐Lin Zhuang, Jiang‐Wei Zhang, Fang Luo, more

Angewandte Chemie > 135 > 6 > n/a - n/a

We explored a co‐dissolved strategy to embed mono‐dispersed Pt center into V₂O₅ support via dissolving [PtV₉O₂₈]⁷⁻ into [V₁₀O₂₈]⁶⁻ aqueous solution. The uniform dispersion of [PtV₉O₂₈]⁷⁻ in [V₁₀O₂₈]⁶⁻ solution allows [PtV₉O₂₈]⁷⁻ to be surrounded by [V₁₀O₂₈]⁶⁻ clusters via a freeze‐drying process. The V centers in both [PtV₉O₂₈]⁷⁻ and [V₁₀O₂₈]⁶⁻ were converted into V₂O₅ via a calcination process to...

article

Co‐Dissolved Isostructural Polyoxovanadates to Construct Single‐Atom‐Site Catalysts for Efficient CO₂ Photoreduction

Yu‐Jie Wang, Gui‐Lin Zhuang, Jiang‐Wei Zhang, Fang Luo, more

Angewandte Chemie International Edition > 62 > 6 > n/a - n/a

article

W Single‐Atom Catalyst for CH₄ Photooxidation in Water Vapor

Ye Wang, Jiangwei Zhang, Wen‐Xiong Shi, Gui‐Lin Zhuang, more

Advanced Materials > 34 > 33 > n/a - n/a

Solar‐driven high‐efficiency and direct conversion of methane into high‐value‐added liquid oxygenates against overoxidation remains a great challenge. Herein, facile and mass fabrication of low‐cost tungsten single‐atom photocatalysts is achieved by directly calcining urea and sodium tungstate under atmosphere (W‐SA‐PCN‐m, urea amount m = 7.5, 15, 30, and 150 g). The single‐atom photocatalysts can...

article

Switching Excited State Distribution of Metal–Organic Framework for Dramatically Boosting Photocatalysis

Song Guo, Li‐Hui Kong, Ping Wang, Shuang Yao, more

Angewandte Chemie > 134 > 30 > n/a - n/a

Photosensitization associated with electron/energy transfer represents the central science of natural photosynthesis. Herein, we proposed a protocol to dramatically improve the sensitizing ability of metal–organic frameworks (MOFs) by switching their excited state distribution from ³MLCT (metal‐to‐ligand charge transfer) to ³IL (intraligand). The hierarchical organization of ³IL MOFs and Co/Cu catalysts...

article

Switching Excited State Distribution of Metal–Organic Framework for Dramatically Boosting Photocatalysis

Song Guo, Li‐Hui Kong, Ping Wang, Shuang Yao, more

Angewandte Chemie International Edition > 61 > 30 > n/a - n/a

article

High‐Efficiency Generation of Flat High‐Order Sidebands in a Gently Modulating Optomechanical System

Jun‐Hao Liu, Ya‐Fei Yu, Jin‐Dong Wang, Zhi‐Ming Zhang

Annalen der Physik > 534 > 2 > n/a - n/a

The high‐order sideband generation in a gently modulating optomechanical system, which consists of a standard optomechanical system driven by a mildly amplitude modulated field (MAMF) is investigated. It is found that the sideband generation can be effectively optimized by choosing an appropriate component number N of the MAMF, and this scheme can generate more and flatter high‐order sidebands with...

article

Construction of Low‐Cost Z‐Scheme Heterostructure Cu₂O/PCN for Highly Selective CO₂ Photoreduction to Methanol with Water Oxidation

Zhi‐Yuan Tian, Li‐Hui Kong, Ye Wang, Hong‐Juan Wang, more

Small > 17 > 44 > n/a - n/a

Solar‐driven CO₂ reaction with water oxidation into alcohols represents a promising approach to achieve real artificial photosynthesis. However, rapid recombination of photogenerated carriers seriously restricts the development of artificial photosynthesis. Herein, a facile method is explored to construct low‐cost Z‐Scheme heterostructure Cu₂O/polymeric carbon nitride (PCN) by in situ growth of Cu...

article

Charge Transfer from Donor to Acceptor in Conjugated Microporous Polymer for Enhanced Photosensitization

Yuan‐Zhao Peng, Guang‐Chen Guo, Song Guo, Li‐Hui Kong, more

Angewandte Chemie > 133 > 40 > 22233 - 22240

Photosensitization associated with light absorption and energy/electron‐transfer represents the central processes for photosynthesis. However, it's still a challenge to develop a heavy‐atom‐free (HAF) strategy to improve the sensitizing ability of polymeric photosensitizers. Herein, we propose a new protocol to significantly improve the photosensitization by decorating mother conjugated microporous...

article

Charge Transfer from Donor to Acceptor in Conjugated Microporous Polymer for Enhanced Photosensitization

Yuan‐Zhao Peng, Guang‐Chen Guo, Song Guo, Li‐Hui Kong, more

Angewandte Chemie International Edition > 60 > 40 > 22062 - 22069

article

Strong Visible‐Light‐Absorbing Cuprous Sensitizers for Dramatically Boosting Photocatalysis

Kai‐Kai Chen, Song Guo, Heyuan Liu, Xiyou Li, more

Angewandte Chemie > 132 > 31 > 13051 - 13057

Developing strong visible‐light‐absorbing (SVLA) earth‐abundant photosensitizers (PSs) for significantly improving the utilization of solar energy is highly desirable, yet it remains a great challenge. Herein, we adopt a through‐bond energy transfer (TBET) strategy by bridging boron dipyrromethene (Bodipy) and a Cu^I complex with an electronically conjugated bridge, resulting in the first SVLA Cu^I...

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INFONA - science communication portal

Search results for: Zhi-Ming Zhang

Single Dispersion of Fe(H₂O)₂‐Based Polyoxometalate on Polymeric Carbon Nitride for Biomimetic CH₄ Photooxidation

Single‐cluster Functionalized TiO₂ Nanotube Array for Boosting Water Oxidation and CO₂ Photoreduction to CH₃OH

Single‐cluster Functionalized TiO₂ Nanotube Array for Boosting Water Oxidation and CO₂ Photoreduction to CH₃OH

Building Co₁₆‐N₃‐Based UiO‐MOF to Expand Design Parameters for MOF Photosensitization

Building Co₁₆‐N₃‐Based UiO‐MOF to Expand Design Parameters for MOF Photosensitization

Water‐Mediated Selectivity Control of CH₃OH versus CO/CH₄ in CO₂ Photoreduction on Single‐Atom Implanted Nanotube Arrays

Identification of Crucial Photosensitizing Factors to Promote CO₂‐to‐CO Conversion

Identification of Crucial Photosensitizing Factors to Promote CO₂‐to‐CO Conversion

Spin Manipulation in a Metal–Organic Layer through Mechanical Exfoliation for Highly Selective CO₂ Photoreduction

Spin Manipulation in a Metal–Organic Layer through Mechanical Exfoliation for Highly Selective CO₂ Photoreduction

Co‐Dissolved Isostructural Polyoxovanadates to Construct Single‐Atom‐Site Catalysts for Efficient CO₂ Photoreduction

Co‐Dissolved Isostructural Polyoxovanadates to Construct Single‐Atom‐Site Catalysts for Efficient CO₂ Photoreduction

W Single‐Atom Catalyst for CH₄ Photooxidation in Water Vapor

Switching Excited State Distribution of Metal–Organic Framework for Dramatically Boosting Photocatalysis

Switching Excited State Distribution of Metal–Organic Framework for Dramatically Boosting Photocatalysis

High‐Efficiency Generation of Flat High‐Order Sidebands in a Gently Modulating Optomechanical System

Construction of Low‐Cost Z‐Scheme Heterostructure Cu₂O/PCN for Highly Selective CO₂ Photoreduction to Methanol with Water Oxidation

Charge Transfer from Donor to Acceptor in Conjugated Microporous Polymer for Enhanced Photosensitization

Charge Transfer from Donor to Acceptor in Conjugated Microporous Polymer for Enhanced Photosensitization

Strong Visible‐Light‐Absorbing Cuprous Sensitizers for Dramatically Boosting Photocatalysis

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