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Magnetoelectric studies on BaTi1−xSnxO3/NiFe2O4 (x = 0.07, 0.08, 0.09 and 0.10) lead-free bilayer laminated composites were investigated at 1 kHz and resonance frequencies. The pure phase formation of BaTi1−xSnxO3 and NiFe2O4 samples was confirmed by X-ray diffraction technique. The ferroelectric BaTi1−xSnxO3 layers of different compositions having large piezocoefficient were used for the ME studies...