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Photocatalytic CO2 reduction to high‐value chemicals is an attractive approach to mitigate climate change, but it remains a great challenge to produce a specific product selectively by IR light. Hence, UiO‐66/Co9S8 composite is designed to couple the advantages of metallic photocatalysts and porous CO2 adsorbers for IR‐light‐driven CO2‐to‐CH4 conversion. The metallic nature of Co9S8 endows UiO‐66/Co...