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In the active site of several copper monooxygenases, thioether residues are coordinated through the sulfur atom, e. g. dopamine‐β‐monooxygenase (DβM). The reaction of dioxygen with a series of copper(I) complexes with thioether groups in tripodal ligands based on either derivatives of tris(2‐pyridylmethyl)amine (TMPA) or a guanidine system were investigated by low‐temperature stopped‐flow measurements...