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A series of five and six‐membered C‐C bonded energetic materials (2–7) based on a combination of imidazole‐triazine and triazole‐triazine backbones were designed, synthesized, and characterized using NMR, IR, Mass spectrometry, and TGA‐DSC studies. Further, the structure of compound 4 was supported by single‐crystal X‐ray analysis. All the newly synthesized energetic compounds exhibit good density,...