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Rate coefficients have been measured for Cl atom reactions under ambient conditions with acetone and four cyclic ketones. Cl was generated by UV photolysis of Cl2, and other species were monitored by FT‐IR spectroscopy. The measurements yield k(Cl + acetone) = (2.0 ± 0.7) × 10−12, k(Cl + cyclobutanone) = (10.1 ± 0.8) × 10−11, k(Cl + cycloheptanone) = (24.0 ± 2.3) × 10−11, k(Cl + 2‐methyl cyclopentanone)...