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Noncentrosymmetric ternary and quaternary chalcogenides are studied as promising nonlinear optical (NLO) materials in the mid‐infrared region. Here, we report the synthesis of a new material BaCu2SiS4 in the AIIBI2MIVQ4 family (A=divalent metal; B=monovalent metal; M=tetrel, Q=chalcogen), and discuss its crystal structure, thermal stability, optical behavior, and electronic structure. BaCu2SiS4 crystallizes...
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