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A series of different molecular weight Polycyclooctene(PCOE) rubber were synthesized via ROMP with G2 catalyst and Iso‐polypropylene (iPP), PCOE and high density polyethylene (HDPE) blends were prepared by micro twin‐screw extruder. The effects of PCOE molecular weight and content were investigated by studying the thermal, rheological and mechanical properties of the blends. We observed that the low...